Continuous magnetic phase transition in artificial square ice
Sendetskyi, OlesLaboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, Switzerland - Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Villigen PSI, Switzerland
Scagnoli, ValerioLaboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, Switzerland - Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Villigen PSI, Switzerland
Leo, NaëmiLaboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, Switzerland - Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Villigen PSI, Switzerland
Anghinolfi, LucaLaboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, Switzerland - Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Villigen PSI, Switzerland - Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, Villigen PSI, Switzerland
Alberca, AuroraSwiss Light Source, Paul Scherrer Institute, Villigen PSI, Switzerland - Department of Physics and Fribourg Centre for Nanomaterials, University of Fribourg, Switzerland
Lüning, JanSorbonne Universités, UPMC Univ Paris 06, Paris, France - CNRS, UMR 7614, LCPMR, 75005 Paris, France
Staub, UrsSwiss Light Source, Paul Scherrer Institute, Villigen PSI, Switzerland
Derlet, Peter MichaelCondensed Matter Theory Group, Paul Scherrer Institute, Villigen PSI, Switzerland
Heyderman, Laura JaneLaboratory for Mesoscopic Systems, Department of Materials, ETH Zurich, Switzerland - Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Villigen PSI, Switzerland
Physical Review B. - 2019, vol. 99, no. 21, p. 214430
English
Critical behavior is very common in many fields of science and a wide variety of many- body systems exhibit emergent critical phenomena. The beauty of critical phase transitions lies in their scale-free properties, such that the temperature dependence of physical parameters of systems differing at the microscopic scale can be described by the same generic power laws. In this work we establish the critical properties of the antiferromagnetic phase transition in artificial square ice, showing that it belongs to the two-dimensional Ising universality class, which extends the applicability of such concepts from atomistic to mesoscopic magnets. Combining soft x-ray resonant magnetic scattering experiments and Monte Carlo simulations, we characterize the transition to the low-temperature long-range order expected for the artificial square-ice system. By measuring the critical scattering, we provide direct quantitative evidence of a continuous magnetic phase transition, obtaining critical exponents which are compatible with those of the two-dimensional Ising universality class. In addition, by varying the blocking temperature relative to the phase transition temperature, we demonstrate its influence on the out-of-equilibrium dynamics due to critical slowing down at the phase transition.