Journal article

High energy resolution off-resonant spectroscopy: A review

  • Błachucki, Wojciech Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw, Poland
  • Hoszowska, Joanna Department of Physics, University of Fribourg, Switzerland
  • Dousse, Jean-Claude Department of Physics, University of Fribourg, Switzerland
  • Kayser, Yves Physikalisch-Technische Bundesanstalt (PTB), Berlin, Germany
  • Stachura, Regina Institute of Physics, Jan Kochanowski University, Kielce, Poland
  • Tyra³a, Krzysztof Institute of Physics, Jan Kochanowski University, Kielce, Poland
  • Wojtaszek, Klaudia Institute of Physics, Jan Kochanowski University, Kielce, Poland
  • Sá, Jacinto Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw, Poland - Department of Chemistry, Uppsala University, Uppsala , Sweden
  • Szlachetko, Jakub Institute of Physical Chemistry, Polish Academy of Sciences, Warsaw, Poland - Institute of Physics, Jan Kochanowski University, Kielce, Poland
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    01.10.2017
Published in:
  • Spectrochimica Acta Part B: Atomic Spectroscopy. - 2017, vol. 136, p. 23–33
English We review the high energy resolution off-resonant spectroscopy (HEROS) technique. HEROS probes the unoccupied electronic states of matter in a single-shot manner thanks to the combination of off-resonant excitation around atomic core states using wavelength dispersive X-ray detection setups. In this review we provide a general introduction to the field of X-ray spectroscopy together with the specification of the available X-ray techniques and X-ray methodologies. Next, the theoretical description of the HEROS approach is introduced with a special focus on the derivation of the X- ray emission and X-ray absorption correspondence relation at off-resonant excitation conditions. Finally, a number of experimental HEROS reports are reviewed in the field of chemistry and material science. We emphasize the applicability of HEROS to pulsed X-ray sources, like X-ray free electron lasers, and support the review with experimental examples. The review is complemented with perspectives on and possible further applications of the HEROS technique to the field of X-ray science.
Faculty
Faculté des sciences et de médecine
Department
Département de Physique
Language
  • English
Classification
Physics
License
License undefined
Identifiers
Persistent URL
https://folia.unifr.ch/unifr/documents/306494
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