Light Management: A Key Concept in High-Efficiency Perovskite/Silicon Tandem Photovoltaics.
- Jacobs DA Research School of Electrical, Energy and Materials Engineering , Australian National University , Canberra 2600 , Australia.
- Langenhorst M Institute of Microstructure Technology , Karlsruhe Institute of Technology , 76344 Eggenstein-Leopoldshafen , Karlsruhe , Germany.
- Sahli F Ecole Polytechnique Fédérale de Lausanne (EPFL), Institute of Microengineering (IMT) Photovoltaics and Thin-Film Electronics Laboratory (PV-Lab) , 2002 Neuchâtel , Switzerland.
- Richards BS Institute of Microstructure Technology , Karlsruhe Institute of Technology , 76344 Eggenstein-Leopoldshafen , Karlsruhe , Germany.
- White TP Research School of Electrical, Energy and Materials Engineering , Australian National University , Canberra 2600 , Australia.
- Ballif C Ecole Polytechnique Fédérale de Lausanne (EPFL), Institute of Microengineering (IMT) Photovoltaics and Thin-Film Electronics Laboratory (PV-Lab) , 2002 Neuchâtel , Switzerland.
- Catchpole KR Research School of Electrical, Energy and Materials Engineering , Australian National University , Canberra 2600 , Australia.
- Paetzold UW Institute of Microstructure Technology , Karlsruhe Institute of Technology , 76344 Eggenstein-Leopoldshafen , Karlsruhe , Germany.
- 2019-05-24
Published in:
- The journal of physical chemistry letters. - 2019
English
The remarkable recent progress in perovskite photovoltaics affords a novel opportunity to advance the power conversion efficiency of market-dominating crystalline silicon (c-Si) solar cells. A severe limiting factor in the development of perovskite/c-Si tandems to date has been their inferior light-harvesting ability compared to single-junction c-Si solar cells, but recent innovations have made impressive headway on this front. Here, we provide a quantitative perspective on future steps to advance perovskite/c-Si tandem photovoltaics from a light-management point of view, addressing key challenges and available strategies relevant to both the 2-terminal and 4-terminal perovskite/c-Si tandem architectures. In particular, we discuss the challenge of achieving low optical reflection in 2-terminal cells, optical shortcomings in state-of-the-art devices, the impact of transparent electrode performance, and a variety of factors which influence the optimal bandgap for perovskite top-cells. Focused attention in each of these areas will be required to make the most of the tandem opportunity.
- Language
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- English
- Open access status
- green
- Identifiers
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- DOI 10.1021/acs.jpclett.8b03721
- PMID 31117674
- Persistent URL
- https://folia.unifr.ch/global/documents/282246
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