High Temperature-Stable Perovskite Solar Cell Based on Low-Cost Carbon Nanotube Hole Contact.
Journal article

High Temperature-Stable Perovskite Solar Cell Based on Low-Cost Carbon Nanotube Hole Contact.

  • Aitola K Department of Chemistry - Ångström Laboratory Physical Chemistry, Uppsala University, Box 523, 75120, Uppsala, Sweden.
  • Domanski K Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, École Polytechnique de Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
  • Correa-Baena JP Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, MA, 02139, USA.
  • Sveinbjörnsson K Department of Chemistry - Ångström Laboratory Physical Chemistry, Uppsala University, Box 523, 75120, Uppsala, Sweden.
  • Saliba M Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, École Polytechnique de Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
  • Abate A Adolphe Merkle Institute, University of Fribourg, CH-1700, Fribourg, Switzerland.
  • Grätzel M Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, École Polytechnique de Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
  • Kauppinen E Department of Applied Physics, Aalto University, P.O. Box 15100, 00076, Aalto, Finland.
  • Johansson EMJ Department of Chemistry - Ångström Laboratory Physical Chemistry, Uppsala University, Box 523, 75120, Uppsala, Sweden.
  • Tress W Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, École Polytechnique de Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
  • Hagfeldt A Laboratory of Photomolecular Science, Institute of Chemical Sciences and Engineering, École Polytechnique Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
  • Boschloo G Department of Chemistry - Ångström Laboratory Physical Chemistry, Uppsala University, Box 523, 75120, Uppsala, Sweden.
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  • 2017-02-24
Published in:
  • Advanced materials (Deerfield Beach, Fla.). - 2017
English Mixed ion perovskite solar cells (PSC) are manufactured with a metal-free hole contact based on press-transferred single-walled carbon nanotube (SWCNT) film infiltrated with 2,2,7,-7-tetrakis(N,N-di-p-methoxyphenylamine)-9,90-spirobifluorene (Spiro-OMeTAD). By means of maximum power point tracking, their stabilities are compared with those of standard PSCs employing spin-coated Spiro-OMeTAD and a thermally evaporated Au back contact, under full 1 sun illumination, at 60 °C, and in a N2 atmosphere. During the 140 h experiment, the solar cells with the Au electrode experience a dramatic, irreversible efficiency loss, rendering them effectively nonoperational, whereas the SWCNT-contacted devices show only a small linear efficiency loss with an extrapolated lifetime of 580 h.
Language
  • English
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closed
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Persistent URL
https://folia.unifr.ch/global/documents/25579
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